Angeo 32 41 2014
Angeo 32 41 2014
Angeo 32 41 2014
Received: 19 July 2013 – Revised: 28 October 2013 – Accepted: 16 December 2013 – Published: 28 January 2014
1–4 W m−2 ) mainly occurred in heavily industrialized re- response to global dimming (Roderick and Farquhar, 2002;
gions (Wild, 2012a). In some non-industrialized countries Liu et al., 2004; Qian et al., 2006).
(e.g., India and Zimbabwe), dimming is still being experi- This review therefore attempts to conclusively address the
enced (Wild et al., 2005). A similar trend was observed in evidence of dimming and brightening in China, determine
sunshine hours (SH) in the contiguous United States (Angell the primary driver from the two most likely candidates of
and Korshover, 1978), western Europe (Sanchez-Lorenzo et clouds and aerosols, and discuss the possible implications of
al., 2008) and Japan (Stanhill and Cohen, 2008) since the dimming and brightening for pan evaporation processes.
1980s and earlier. SH, which quantifies the length of time
with direct solar radiation ≥ 120 W m−2 in each day, is a
widely used proxy for SSR. 2 Evidence of dimming and brightening in China
Two fundamental ways to change SSR include (1) exter-
nally changing incoming solar radiation by changing Earth’s 2.1 Dimming and brightening in surface solar radiation
orbital parameters or solar output; and (2) internally chang-
ing the reflected fraction of solar radiation via changing The national solar radiation monitoring network, consisting
cloud characteristics, radiatively active gases (especially wa- of 122 stations in mainly urban or suburb regions across
ter vapor), aerosol masses and optical properties or surface China (Fig. 1), was established in 1957 (Liang and Xia,
albedo (IPCC, 2007; Wild, 2009). The effects of Earth’s 2005). The solar radiation instruments were later updated.
orbital parameters and water vapor on observed decadal Before 1993, solar radiation instruments were developed af-
variations in SSR are largely negligible. This is because ter the models of the former Soviet Union. These instru-
Earth’s orbital parameters vary substantially on geologi- ments included the Yanishevsky thermoelectric pyranometer
cal timescales greater than 10 000 yr, and the magnitude of for measuring SSR and diffuse solar radiation (DfSR) and the
change in water vapor in recent decades is insufficient for Yanishevsky thermoelectric actinometer for measuring direct
a significant fluctuation in SSR (Hoyt and Schatten, 1993; solar radiation (DiSR) (Xia, 2010a; Ye et al., 2010; Tang et
Ramanathan and Vogelmann, 1997; Solomon et al., 2010). al., 2011), with respective error estimates of ≤5 % and ≤3 %
Based on IPCC (2007) estimates, among all the negative (Shi et al., 2008). China started making its own instruments
radiative forcings resulted from human activities (e.g., to- after 1993 and replaced the SSR/DfSR recorders with the
tal aerosol, surface albedo and ozone), aerosols induce the DFY-4 pyranometer and the DiSR recorder with the DFY-3
largest effect. To a great extent, therefore, global dimming pyrheliometer (Xia, 2010a; Ye et al., 2010; Tang et al., 2011),
and brightening should be caused by clouds and aerosols, with errors not exceeding 5 % and 2 %, respectively (Shi et
which respectively denote the impact of climate change and al., 2008). Data recorded by the instruments are governed by
anthropogenic disturbances (Shi et al., 2008; Gilgen et al., China Meteorological Administration (CMA) and are avail-
2009; Ohmura, 2009; Streets et al., 2009; Wild, 2009; Xia, able at China Meteorological Data Sharing Service System
2010b). So far, it remains inconclusive whether clouds or (CMDS, http://cdc.cma.gov.cn/). Preliminary quality checks
aerosols are the main driver of recent changes in SSR. In- are also performed by CMA to ensure that both DiSR and
creasing studies tend to support the concept that while clouds DfSR are lower than SSR for daily data (see interpretation
effectively modulate SSR at annual scale, pollution-related of documented data sets). However, the simple quality con-
aerosols determine the variability of SSR at decadal scale trol criterion could not eliminate the potential accuracy issues
(Qian et al., 2006, 2007; Wang et al., 2012b; Wang et al., related with instrument change, artificial operational factors
2013). Generally, global and regional average trends in SSR and station location change (Shi et al., 2008). In an attempt to
are in line with those in anthropogenic aerosol emissions resolve this issue, Shi et al. (2008) introduced a set of quality
(Stern, 2006; Streets et al., 2006, 2009; Wild, 2012a). assessment (QA) algorithms, including a physical threshold
Variations in SSR could alter the latent heat flux and evap- test (QA1), a global radiation sunshine duration test (QA2),
oration energy equivalent, which in turn changes the inten- and a standard deviation test applied to time series of annu-
sity of the hydrological cycle (Ramanathan et al., 2001; Wild, ally averaged solar global radiation (QA3). Recently, Tang
2009, 2012a; Wild and Liepert, 2010). Since the 1950s, de- et al. (2010) presented a new quality control scheme that in-
clines in pan evaporation have been detected not only in the cludes two physical threshold tests, a test to remove monthly-
Northern Hemisphere (Peterson et al., 1995; Chattopadhyay mean values with evident systematic and operational errors,
and Hulme, 1997; Liu et al., 2004), but also in the Southern and a test to eliminate the data with more insidious errors
Hemisphere (Roderick and Farquhar, 2005; Rayner, 2007). using the artificial neural network (ANN) method. Scientific
This is contrary to the expectation that global warming in- results based on screened data by these strict quality controls
creases evaporation from terrestrial water bodies. This dis- have proven to be highly reliable.
crepancy between observations and expectations is termed Consistent with the global SSR trend, there is abundant ev-
“pan evaporation paradox” (Brutsaert and Parlange, 1998). idence of the “from dimming to brightening” transition in the
Increasingly, research proposes that the downward pan evap- SSR trend in China in the past half century (Wild et al., 2005;
oration trend is rather not a real paradox but simply a Shi et al., 2008; Norris and Wild, 2009; Ohmura, 2009; Wang
Number
Reference 1950s 1960s 1970s 1980s 1990s 2000s
of sites
Che et al. ( 2005) 64 –4.5
# –9.1 # #
Liang and Xia (2005) 42 –4.9b
Qian et al. (2006) 85 –3.1
Yang et al. (2007) 60 –3.4a
Shi et al. (2008) 72 –3.8b
# –7b 2.7b
Norris and Wild (2009) 23 –11 4
Ohmura (2009) 66 –12 #
Wang et al. (2009) 30 –8.8a 1.4a
Tang et al. (2011) 96 –2.3
–2.5 0.4
Wild et al. (2012a) # –7 3 –4
Yang and Yang (2012) 54 –4.5
Table 2. Regional characteristics of surface solar radiation trends in China for the 1960s–1980s (dimming phase) and 1990s–2000s (bright-
ening phase).
1960s–1980s 1990s–2000s
Number
Reference of sites Strong dimming Slight dimming Dimming Brightening
Liu et al. (2004) 85 Southeastern China
Liang and Xia (2005) 42 Southern and eastern China
Ohmura (2006) 66 Southeastern China Northwestern China Northern China Southeastern China
Qian et al. (2006) 85 Central, eastern and southern China
Yang et al. (2007) 60 Eastern China Northeastern China Northern China, Southeastern and southwestern China,
and Yunnan area and northern Xinjiang Tibetan Plateau
Shi et al. (2008) 72 Southern China Northeastern and western China
Xia (2010a) 45 Southeastern China Southwestern China Northern China Southern China
Wang et al. (2011) 40 Central and southern China Western arid/semi-arid Northern China and western Southern and southwestern
regions, northeastern China arid/semi-arid regions China, Tibetan Plateau
Wild and Schmucki (2011) 13 Southeastern China Northwestern China Northwestern China Southeastern China
181 7.0 1960s–1990s (Che et al., 2005; Liang and Xia, 2005; Shi
Surface solar radiation (W m )
(a) (b)
–2
179
et al., 2008) and moderately increases thereafter (Wen et
Sunshine hours (h d )
6.6
–1
177
175 6.2
al., 2008; Zhao et al., 2009). The geographical distribution
173 0.04
−0.002
of the variation in DiSR is very similar to that in SSR.
5.8
171
−0.25* −0.028*
It primarily declines in southern and eastern China but at
169
167
5.4 much smaller rate in western and northeastern China (Liang
165 5.0 and Xia, 2005; Shi et al., 2008; Zhao et al., 2009). Recent
1960 1966 1972 1978 1984 1990 1996 2002 2008 1960 1966 1972 1978 1984 1990 1996 2002 2008
1800 0.35 110 studies on seasonal trends in DiSR have drawn almost
(c) (d)
1750
0.32 100 the opposite conclusions. Based on estimated DiSR from
Pan evaporation (mm)
1700
0.003*
SH data obtained from 70 stations across China, Zhao et
7.9* 0.29 90
AOD
1650
0.26 80
1600 summer, followed by spring, autumn and winter for the
−5.4* 0.23 −1.844* 70 period 1960–2005. However, based on observed DiSR data
1550
1500 0.20 60
from 14 stations across China, Ma et al. (2011) observed
1960 1966 1972 1978 1984 1990 1996 2002 2008 1960 1966 1972 1978 1984 1990 1996 2002 2008
Year Year that DiSR decline is most obvious in winter and autumn
936
and insignificant in spring and summer for the period
Fig. 2. Time series comparisons of annually averaged surface solar 1961–2009. The inconsistency of the results could be due to
937 Fig. 2. Time series comparisons of annually averaged surface solar radiation (A, data from
radiation (a, data from Tang et al., 2011), sunshine hours (b, data differences in the number of samples and length of periods
938 Tang et al. (2011)), sunshine hours (B, data from Wang et al. (2013)), pan evaporation (C,
939
from Wang et al., 2013), pan evaporation (c, data from Liu et al.,
data from Liu et al. (2011a)), AOD and API (D, data from Streets et al. (2008) and Wang et al. of the analyses, as well as limitations in surface observation
9402011a), AOD
(2013) for andand
1980−2000 API (d, data
2001−2011, from Streets
respectively) over Chinaetforal.,
the2008 and Wang
1960s−2000s. Blue et
of DiSR in China.
941al.,lines
2013
denotefor 1980–2000
linear and
trends in dimming phase2001–2011, respectively)
and red lines indicate over China
linear trends in brightening
942forphase.
DfSR shows a less pronounced trend of decline in China,
the Values
1960s–2000s. Blue
are trend slopes and lines
asterisks denote
denote linear
a significant trends
trend at the 95% in dimming
confidence
943phase
level. and red lines indicate linear trends in brightening phase. Val- which is at the average rate of 0.92–0.95 % decade−1
ues are trend slopes and asterisks denote a significant trend at the (about 0.72 W m−2 decade−1 ) during the 1960s–1990s (Che
95 % confidence level. et al., 2005; Shi et al., 2008). Annual average DfSR varies
smoothly before 1980, significantly declines in 1981–1990
(Che et al., 2005), and then rebounds till 2010 (Ren et al.,
dimming in China around 2000. All of these results come to 2013). However, Qian et al. (2007) noted a steady DfSR in-
an agreement that brightening in China is not as significant
36 crease in China under cloud-free skies for the period 1961–
as in industrialized nations. 1992. DfSR depicts a more complex and heterogeneous spa-
tial pattern. While in the 1960s–1990s sites with downward
2.2 Dimming and brightening in direct and diffuse solar trends are mainly in northwestern China and the Tibetan
radiation Plateau, those with upward trends are largely in coastal areas
and the middle and lower reaches of Yellow River (Liang and
SSR is total shortwave radiation, constituting the direct com- Xia, 2005; Shi et al., 2008; Ma et al., 2011). From 1980, the
ponent from the Sun (DiSR) and diffuse component from most evident increase and decrease in DfSR are respectively
the sky (DfSR), incident on the horizontal surface (Xia et in the Tibetan Plateau and northwestern China (Ren et al.,
al., 2006; Qian et al., 2007; Wild, 2009). Variations in SSR 2013). No obvious seasonal trend in DfSR is detected since
closely correspond with the changes in the trend and magni- 1960 (Liang and Xia, 2005; Ma et al., 2011). With the ex-
tude of DiSR and DfSR. ception of spring, DfSR increases in trend in all the seasons
In China, DiSR decreases in the range of 7.5– during the period 1981–2010 (Ren et al., 2013).
8.6 % decade−1 (about 6.6 W m−2 decade−1 ) during
Table 3. Correlation coefficients between radiative (SSR, surface solar radiation; SH, sunshine hours) and meteorological (TCC, total cloud
cover; LCC, low cloud cover; WS, wind speed; VAP, water vapor pressure; RH, relative humidity; P , precipitation; Epan , pan evaporation)
variables.
Number
Reference Study area of sites Period TCC LCC WS VAP RH P Epan
SSR Qian et al. (2006) Whole China 85 1955–2000 0.57c
Xu et al. (2006) Whole China 305 1969–2000 0.714b
Wang et al. (2010) Southeastern China 85 1961–2008 −0.488b −0.727b
Zheng et al. (2011) Yunnan–Guizhou Plateau 8 1961–2005 −0.880b 0.237a −0.526b
SH Ren and Guo (2006) Whole China 600 1956–2000 0.75b
Du et al. (2007) Tibet 25 1971–2005 −0.052c −0.373c −0.749c −0.522c
Shen and Sheng (2008) Whole China 472 1957–2001 0.61b
Cong et al. (2009) Whole China 317 1956–2005 0.75a
Yang et al. (2009a) Northern China 81 1965–1999 0.66b –0.64b –0.48b
Xia (2010b) Whole China 618 1955–2005 0.23 −0.52a
You et al. (2010) Eastern and central Tibetan Plateau 71 1961–2005 −0.07 −0.76a −0.65 −0.61a −0.51a
Li et al. (2011) Low-altitude belt of southern China 147 1961–2005 −0.47b −0.90b
Yu et al. (2011) Whole China 194 1951–2009 0.76b −0.27a
Li et al. (2012) Southwestern China 111 1961–2009 −0.34a 0.58a −0.32a −0.29a
Yang et al. (2012b) Southwestern China 110 1969–2009 0.46a
a p < 0.05, b p < 0.01, c not given.
forcings (Charlson et al., 1992; Ramanathan et al., 2001). site (70 km southeast of Beijing), Li et al. (2007b) de-
Direct radiative forcing refers to the scattering (primarily tected that high aerosol loading resulted in a very large
by sulfate, nitrate, and organic carbon aerosols) and/or ab- aerosol radiative effect at the surface (the annual mean value
sorption (primarily by BC aerosols) of solar radiation by the equals −24.1 W m−2 ) from September 2004 to Septem-
nature of aerosol composition (IPCC, 2007; Myhre, 2009; ber 2005; only moderately lower than the cloud radiative
Dwyer et al., 2010; Satheesh, 2012). Indirect radiative forc- effect (−41.0 W m−2 ). At the Taihu site (100 km west of
ing is caused by aerosols acting as cloud condensation nuclei Shanghai), Xia et al. (2007b) noted that heavy aerosol load-
(CNN) and ice nuclei, which in turn influence cloud radiative ing resulted in −45.5 W m−2 and −112.6 W m−2 reductions
properties and lifetimes (Charlson et al., 1992; Ramanathan in SSR and DiSR while 67.1 W m−2 more DfSR reached
et al., 2001; IPCC, 2007). All the aerosol radiative forcings Earth’s surface from September 2005 to August 2006. The
act towards reducing SSR and SH. Moreover, aerosols could annual mean aerosol direct radiative forcing at the surface
have semi-direct radiative forcing by inhibiting cloud forma- amounted to −38.4 W m−2 . At the Liaozhong site, a subur-
tion or dissolving existing clouds as absorbing aerosols in ban region in northeastern China, Xia et al. (2007a) estimated
heavily polluted regions could heat up and stabilize the atmo- that aerosols reduced SSR by 30 W m−2 day−1 from April to
sphere (Wild, 2009). This could partially counteract aerosol- June 2005.
induced dimming in heavily polluted areas for reduced cloud Aerosol optical depth (AOD) and air pollution index (API)
shading (Wild, 2012a). are the two widely used proxies for aerosols in air quality
Aerosol radiative forcings over the inland areas of China studies (Neha, 2000; He et al., 2002; Li et al., 2003, 2005;
were not quantified until the mid-2000s, when the East Pour-Biazar et al., 2011). AOD (also known as AOT, aerosol
Asian Study of Tropospheric Aerosols: An International Re- optical thickness) measures wavelength-dependent aerosol
gional Experiment (EAST-AIRE) commenced as a USA– extinction in the atmospheric column via remote sensing
China cooperative research endeavor (Li et al., 2007a). It (Bellouin et al., 2005). API is the generalized way of describ-
consists of two baseline observatories established at Xi- ing air quality in China, which is based on 24 h ground-based
anghe and Taihu, a nationwide aerosol observation net- monitoring of mass concentration of three principal air pollu-
work covering 25 stations across China, and two consecu- tants – SO2 , NO2 , and PM10 . API measurements started with
tive IOCs (intensive observation campaigns) conducted in a few stations in 2000 and since then has gradually expanded
the spring of 2005. This was done in March on the ground to 120 environmental monitoring stations, mainly in major
in Xianghe and in April from both aircraft and ground in cities of China (Fig. 1). These data are now available at the
Liaozhong. The EAST-AIRE study primarily aims to ac- China National Environmental Monitoring Center (CNEMC,
quire optical, physical and chemical properties of aerosols http://www.cnemc.cn/), which is managed by the State Envi-
and to understand climatic and environmental effects of the ronmental Protection Bureau (SEPB). Based on the Ambient
aerosol properties. Quantification of aerosol radiative forc- Air Quality Standards, eco-environmental effects of various
ings has therefore been enabled by the simultaneous high- pollutants and their health implications, the API scale (0–
quality observations of aerosol, cloud and radiative quan- 500) corresponds to seven air pollution levels – I (excellent,
tities made in the EAST-AIRE stations. At the Xianghe 0–50), II (good, 51–100), III(1) (slight pollution, 101–150),
where brightening occurs air quality is relatively good. Wang It is worth noting that in spite of the two principal driving
et al. (2012) verified that in cities with average API > 80, the factors (cloud and aerosol), wind also significantly influences
SH decline for the 1960s–2000s is 0.2 h d−1 (2.5 %) stronger SSR and SH. Xu et al. (2006) detected that annual mean wind
than in cities with average daily API ≤ 80. Ground observed speed and surface incoming solar radiation share similar
API and remotely sensed AOD are noted to be strongly cor- decadal trends in China. A significantly positive correlation
related after correction for aerosol seasonal vertical distri- between SSR and WS was also noted by Zheng et al. (2011)
bution and real-time relative humidity (Li et al., 2003; He in the Yunnan–Guizhou Plateau. Among various meteoro-
et al., 2010). The correlation coefficient between AOD and logical parameters, wind speed is most closely correlated
API could improve to 0.54 at 99 % confidence level (Li et with SH in northern China (Yang et al., 2009a), southwest-
al., 2005). ern China (Li et al., 2012; Yang et al., 2012b) and the whole
Figure 2d shows a sharp increase in AOD (simulated using of China (Yu et al., 2011). Corresponding coefficients of the
the GOCART model) over China in the 1980s (Streets et al., observed correlations between SSR/SH and WS are shown
2008), the decade with the strongest decline in SSR and SH in Table 3. Winds could disperse and alter the frequency and
during the last half century. An increase in AOD is especially distribution of air pollutants and aerosol derivatives, thereby
notable in the middle and lower reaches of Yangtze River and indirectly influencing SH and SSR (Lu and Fang, 2002; Xu et
the southern coastal areas (Luo et al., 2000, 2001, 2002; Lu al., 2006; Yang et al., 2009b; Li et al., 2012). In Fig. 5, cities
and Fang, 2002), where strong dimming is prevalent. AOD with relatively good air quality are mainly distributed in the
increases to a peak value of 0.305 in 1996 and declines there- high monsoon wind regions, especially in the tropical and
after (Fig. 2d), corresponding to the transition from dimming subtropical monsoon climate zone (southeastern China). For
to brightening in SSR and SH trends. Following that is an al- the past 50 yr, mean annual wind speed significantly declines
most linear decline in average API in the period 2001–2011 at the rate of 0.1 m s−1 decade−1 in China. This is attributed
(Fig. 2d), especially in spring (Wang et al., 2013), which is to the weakening East Asian monsoon and windbreak effect
consistent with annual and seasonal brightening trends. Simi- of the high-rise buildings, which are quickly constructed in
lar observations were made by Lei et al. (2011a) and Wang et China’s urbanization boom (Z. Wang et al., 2004; Ren et al.,
2005; Zuo et al., 2005; Xu et al., 2006; Cong et al., 2009; spinning up the hydrological cycle (Ramanathan et al., 2001;
Liu et al., 2009; Yin et al., 2010). Wind deceleration could Wild, 2009, 2012a, b).
enhance aerosol concentration in the atmosphere, which in
turn dims SSR and SH in China (Zhao et al., 2010; Yang and 4.2 Implications for pan evaporation
Yang, 2012).
Pan evaporation (Epan ), the most widely used proxy for po-
3.4 Other potential driving factors tential evaporation, measures evaporation in a standard open
pan of water (Wild, 2009). Basically, the potential factors
Other variables also exert non-negligible influences on SSR that influence Epan can be divided into three category terms:
and SH. Despite air pollution, change in surface albedo, thermodynamic term (temperature, sunshine hours and diur-
which is also associated with urbanization, has a negative nal temperature range), aerodynamic term (wind speed and
radiative forcing. Human activities are altering the nature of pressure) and hydrodynamic term (relative humidity, precip-
land cover, especially through changes in croplands, pastures itation and low cloud cover) (Liu et al., 2009; Shen et al.,
and forests, resulting in more reflection of solar radiation 2010). Peterson et al. (1995) attributed the general decline
from Earth’s surface (IPCC, 2007). So far, however, large un- in Epan in the United States and the former Soviet Union
certainties remain in the contributions of changes in surface for the period 1950–1990 to increasing cloudiness. In sub-
albedo to China’s dimming and brightening. sequent studies, Brutsaert and Parlange (1998) proposed that
Water vapor is a strong absorber of solar radiation; i.e., a the observed decline in Epan , which indicated increasing ter-
10 % increase in water vapor attenuates solar radiation by up restrial evaporation, should not be a paradox. Ohumura and
to 0.5 % (Wild, 2009). Wang et al. (2011) showed that SSR Wild (2002) argued that the direction of the Epan trend is not
negatively correlates with near-surface water vapor in most determined by temperature alone. Rayner (2007) identified
regions of China, especially in relatively dry high-latitude wind run (i.e., daily average wind speed) as the dominant fac-
regions. For instance, in the Tibetan Plateau, a higher cor- tor of Epan trends in Australia. Roderick and Farquhar (2002)
relation was noted by Du et al. (2007) and You et al. (2010) theorized the resolution of the pan evaporation paradox by
between SH and water vapor pressure than with other me- explaining how a downward Epan trend could be driven by
teorological variables (Table 3). This suggests that the ef- global dimming. The fact that SSR and Epan trends in China
fect of water vapor on solar radiation largely depends on the have a similar transition in 1990 (Liu et al., 2004; Qian et
background level of water vapor content. Similar variables al., 2006) is further evidence that solar radiation dominantly
with different measurements are relative humidity and pre- controls the recent Epan trend.
cipitation. The interaction of relative humidity and aerosols Figure 2c shows a significant decline in Epan by
influences the development of cloudy conditions (Wang et 54 mm decade−1 in China’s dimming phase (Liu et al.,
al., 2012). Precipitation could wash out aerosols and reduce 2011a), suggesting that solar dimming offsets the effect of
the amount of clouds, which in turn mitigate the effect of increasing air temperature on Epan . The decline in Epan is
aerosols and clouds on SSR and SH (Ramanathan et al., strongest in summer (Ren and Guo, 2006; Liu et al., 2009;
2001). Table 3 shows that relative humidity and precipita- Shen and Sheng, 2009) and in regions around southeastern
tion have a significant negative correlation with SSR/SH in China and the middle and lower reaches of Yangtze River
various regions of China (Yu et al., 2011; Zheng et al., 2011; (Yan et al., 2007; Shen and Sheng, 2008; Liu et al., 2009).
Yang et al., 2012b), especially in the Tibetan Plateau (Du et This corresponds with seasonal and spatial trends in dim-
al., 2007; You et al., 2010) and northern China (Yang et al., ming of SSR and SH. The mean annual Epan in China has
2009a). significantly increased by 79 mm decade−1 since 1992 (Liu
et al., 2011a), consistent with the recovery of solar radiation
4 Hydrological implications of dimming and in the country (Fig. 2). For the period since the mid-1950s,
brightening in China the Epan trend is significantly and positively correlated with
the SSR/SH trend in China (Table 3), with an estimated co-
4.1 Link between radiation balance and efficient ≥ 0.57 (Qian et al., 2006; Ren and Guo, 2006; Shen
hydrological cycle and Sheng, 2008; Cong et al., 2009).
According to Cong et al. (2009, 2010), Epan increases in
Since the process of evaporation requires energy (e.g., latent the north while continues to decrease in the south after 1986;
heat), solar radiation is the principal driver of the global hy- in discordance with the spatial pattern of solar brightening.
drological cycle (Wild and Liepert, 2010). Decreasing SSR This suggests that other factors other than solar radiation also
(i.e., global dimming) could attenuate latent heat of evapo- influence Epan . Cong et al. (2009) and Liu et al. (2011a) reck-
ration and the equivalent global precipitation, thereby spin- oned that increasing Epan since the 1990s is caused by de-
ning down the hydrological cycle. On the other hand, increas- creasing vapor pressure deficit due to strong warming. Wa-
ing SSR (i.e., global brightening) could induce stronger la- ter conditions in different climatic regions and seasons influ-
tent heat of evaporation and more frequent rainfall, thereby ence the sensitivity of Epan to changes in solar radiation (Liu
et al., 2004). Besides this, wind speed is widely regarded and brightening in this region is still under debate. You et
as another important driving factor of the pan evaporation al. (2013) suggested that aerosol is the determinant factor of
paradox in China (Ren et al., 2005; Ren and Guo, 2006; SSR in the Tibetan Plateau. This view is supported by the fact
Cong et al., 2009; Liu et al., 2011a). Shen and Sheng (2008, that aerosol loading is impacted by the long-range transporta-
2009) asserted that thermodynamic and aerodynamic terms tion of anthropogenic aerosols from southern Asia (Xia et al.,
respectively dominate the drop of Epan in eastern and west- 2011) and dust aerosols from the Taklimakan Desert (Xia et
ern China. al., 2008) to the region. However, Yang et al. (2012a) argued
that under low water vapor content and aerosol concentration
in the plateau, water vapor amount and deep cloud cover be-
5 Key regions come the dominant driving factors of SSR. In fact, water va-
por has been verified as a critical regulator of SSR in regions
Southeastern China is the region with the most obvious at high latitudes with dry atmosphere, such as in northeast-
dimming and brightening for the periods 1960s–1980s and ern and northwestern China (Wang et al., 2011). The water
1990s–2000s, respectively (Ohmura, 2006; Xia, 2010a; Wild deficit in northwestern China also increases the sensitivity
and Schmucki, 2011; Wang et al., 2012). The prevailing of Epan to change in SSR, thus the rate of decrease in Epan
climate in the region is tropical and subtropical monsoon is highest in the region (Liu et al., 2004). The pan evapora-
with frequent cloud events, heavy rainfall and strong sun- tion paradox does not exist in northeastern China, because
shine. Since the implementation of the reform and opening- Epan increases with the increasingly warmer climate (Cong
up policy in 1978, this region has experienced fast economic et al., 2009). The dominant climatic factor of the decreasing
growth that has in turn led to a drastic increase in AOD Epan trend in the Tibetan Plateau for the period 1970–2005 is
(Luo et al., 2000, 2001, 2002; Lu and Fang, 2002). Li et wind speed, followed by vapor pressure and SSR (Liu et al.,
al. (2011) showed that increased aerosol loading due to rapid 2011b).
socio-economic development is the driving force behind the
sharp dimming in this region. The latter brightening trend
might be in response to improved air quality. As illustrated 6 Discussions and suggestions for future research
in Fig. 5, the average API level in southeastern China is gen-
erally lower than 70 for the 2000s. Aerosol-linked LCC has It is undisputed that since the 1950s, solar radiation over
been identified as the primary meteorological regulator of China suffers a temporally and spatially prevalent decreas-
SSR and SH in this region (Wang et al., 2010; Li et al., 2011). ing trend. However, the magnitude of China’s dimming esti-
The strongest dimming rate in southeastern China, however, mated in recent studies differs greatly (Che et al., 2005; Shi
was not in phase with the highest Epan decrease in the period et al., 2008; Norris and Wild, 2009; Ohmura, 2009; Wang et
1955–2000. This suggests that plentiful water conditions re- al., 2009; Tang et al., 2011; Wild, 2012a). There is no concor-
duced the sensitivity of Epan to change with SSR (Liu et al., dance in conclusions on the seasonal dimming trends in SSR
2004). (Shi et al., 2008; Wang et al., 2009; Xia, 2010a) and DiSR
Continued dimming since 1990 is prevalent in northern (Zhao et al., 2009; Ma et al., 2011). By contrast, results of
China (Ohmura, 2006; Yang et al., 2007; Xia, 2010a; Wang et estimated SH trends are largely in agreement (Xia, 2010b;
al., 2011, 2013). This region is dominated by the East Asian Zhao et al., 2010; Yu et al., 2011). The uncertainties in solar
monsoon climate of hot, humid, low-latitude western Pacific radiation studies highlight the importance of data quality as-
winds in summer, and cold, dry Siberian winds in winter. In- sessment and control, as erroneous and suspected data could
creased aerosol emissions driven by air pollution have been lead to unreliable and spurious trends. Distinct data sets with
identified by Yang et al. (2009b) as the cause of dimming in varied spatial coverage and timescales could also influence
this region. In Fig. 5, a relatively high level of API could be the consistency of results. In addition, more accurate, higher-
noted. Through interaction with aerosol loading, wind speed order statistical models rather than current linear regressions
exerts the strongest influence on SH in northern China (Yang are needed in trend analysis (Wild, 2009). There is an over-
et al., 2009a). Wind speed, rather than SSR, is also the dom- whelming scientific consensus that increasing anthropogenic
inant factor for decreasing Epan in this region from 1960 to aerosol loading is the most plausible explanation for China’s
the early 1990s (Liu et al., 2011a). A significant wind ef- dimming (Kaiser and Qian, 2002; Che et al., 2005; Qian et
fect is also observed in southwestern China (Li et al., 2012; al., 2006, 2007; Wen et al., 2008; Xia, 2010b). This is further
Yang et al., 2012b), which is a typical monsoonal climate confirmed by the decreasing trend in TCC (Liang and Xia,
region dominated by both the South and East Asian mon- 2005; Xia et al., 2006; Yang et al., 2007; Shen et al., 2008),
soon winds. The pan evaporation paradox is not existent in although cloud changes to some extent account for the dim-
southwestern China, as Epan decreases with decreasing air ming in the Tibetan Plateau (Tang et al., 2011; Yang et al.,
temperature (Cong et al., 2009). 2012a), northwestern China (Xia, 2010a) and most of south-
The smallest mean AOD in China is for the Tibetan ern China (Wang et al., 2010; Li et al., 2011; Zheng et al.,
Plateau region (Xin et al., 2007). Aerosol effect on dimming 2011; Li et al., 2012) (Table 3). A higher dimming rate in
urban regions than in rural regions also reflects the attenua- arid/semi-arid regions of China where the atmosphere is rel-
tion effect of urbanization-induced air pollution on sunlight atively dry, the weakening function of water vapor (rela-
(Li et al., 2012; Wang et al., 2013). So far, proof of aerosol as tive humidity/precipitation) on sunlight is evident (Du et al.,
the prime regulator of China’s dimming largely depends on 2007; You et al., 2010; Wang et al., 2011) (Table 3). In ar-
simple trend comparisons and is insufficient from physical eas with sustained and intensive human activities, radiative
mechanisms. forcing of surface albedo needs consideration.
The solar radiation trend after 1990, however, largely re- Research on hydrological implications of dimming and
mains debatable in China. The latest updates presented that brightening in China is only in its infancy. Despite evapo-
the recent trend in SSR (Tang et al., 2011) and SH (Wang ration, the implications for other hydrological components
et al., 2013) levels off rather than brightening. At a global such as precipitation have seldom been studied in China.
scale, brightening mainly occurs in industrialized regions, Similar to the analyses of the causes of solar dimming and
accompanying a slowdown in anthropogenic emissions and brightening in China, hydrological implications tend to very
economic growth (Wild, 2009, 2012a). Similarly, there was much rely on trend comparisons rather than critical interpre-
improvement of air quality in China in the early 21st cen- tations of physical mechanisms. The main scientific process
tury (Chen et al., 2010; Shaw et al., 2010; Lei et al., 2011b; is that, similar to the solar radiation trend, the Epan trend in
Wang et al., 2012, 2013). In fact, a tremendous effort is ap- China reverses from decreasing to increasing in 1990 (Liu
plied to sustain economic development and intensive envi- et al., 2004; Qian et al., 2006). This evidence further con-
ronmental protection since the start of China’s environmental firms the claim that the pan evaporation paradox could be
protection in the 1970s. Such effort is especially commend- resolved by solar dimming (Roderick and Farquhar, 2002).
able after the 1992 act of sustainable development as a stan- Comparing the dimming phases in Fig. 2a and c, a de-
dard national strategy (Zhang and Wen, 2008). As one of the cline of 2.5 W m−2 decade−1 in SSR is accompanied by a
largest developing countries, China is still in the period of 54 mm decade−1 decline in pan evaporation. For the bright-
rapid economic growth and population expansion. The pos- ening phase, an increase of 0.4 W m−2 decade−1 in SSR is
sibility for renewed dimming cannot be excluded and has accompanied by 79 mm decade−1 increase in pan evapora-
already been discussed in studies of Che et al. (2005) and tion. This suggests that to some extent, solar dimming, but
Wild et al. (2009). It can then be predicted that the future also decreasing wind speed, offsets the effect of warming
solar radiation trend in China could largely depend on the climate on evaporation. This in turn results in a decline in
development of air quality control. On the other hand, the pan evaporation. On the contrast, strong warming with a
possible influence of climate-driven TCC suppression on so- slight increase in solar radiation leads to a more significant
lar recovery after 1990 is non-negligible (Norris and Wild, recovery in pan evaporation for the brightening phase (Liu
2009; Xia, 2010a; Wang et al., 2011). The reversal in SSR et al., 2011a; Wild, 2012a). Assuming that solar dimming
and SH trends could be associated with natural and anthro- and brightening in China are largely driven by anthropogenic
pogenic factors. Being that other radiation factors such as aerosols with possible effects on pan evaporation, hydrolog-
DiSR, DfSR and photosynthetically active radiation (RAR) ical observations and simulations of evaporation could be
are noted to have different environmental implications (Che skewed by air pollution. This aspect of pollution-driven hy-
et al., 2005; Pinker et al., 2005; Zhu et al., 2010), there is a drological processes requires intensive scientific studies for
need for systematic studies on these SSR components. a conclusive clarification. More scientific works are required
Although wind hardly actually changes emission trends to unveil the hydrological implications of solar dimming and
and pollutant sources, the transport of air pollutants is pre- brightening in China.
dominantly controlled by wind speed. In other words, winds
partially determine the residence time, distribution pattern
and pollutant/aerosol concentration in the atmosphere. So far, Acknowledgements. This study is funded by the International Col-
there is no conclusive evidence on the effect of wind speed laborative Project (2012DFG90290) of the Ministry of Science and
Technology and the Basic Research Development Program of China
on SSR and SH under varying air pollution levels. Wind ac-
(2010CB951002). The meteorological and solar radiation data are
celeration could lead to dispersion of aerosols in the source provided by China National Meteorological Information Center
regions, but accumulation of aerosols in the downwind re- (CNMIC). API data are from China National Environmental Mon-
gions. Furthermore, increasing wind speed in the desert and itoring Center (CNEMC). The authors are thankful to Prof. Paolo
Gobi regions could result in more dust aerosols emitted into Michele Ruti and two anonymous reviewers for the invaluable sug-
the atmosphere, which in turn attenuates sunlight. This calls gestions and comments during the review phase of this paper.
for further research on wind speed as a critical driving factor Topical Editor P. M. Ruti thanks X. Xia and one anonymous
of solar radiation to help better understand the cause–effect referee for their help in evaluating this paper.
relationship between air pollution and solar dimming.
The effects of other potential driving factors (water va-
por and surface albedo) on SSR and SH are also non-
negligible in specific conditions. For instance, in western
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